This paper uses the Theory of Majorization to accomplish deterministic transformations of the entangled bipartite pure states in the high dimensional quantum systems. There is a detail process that a 44 dimension quantum system completes the deterministic transformations with a one hundred percent probability by the Theory of Majorization, local operation and classical communication (LOCC) and positive operator valued measure (POVM). By the calculation and theoretical derivation, this entangled pure state deterministic transformations based on the Theory of Majorization can decrease the Von Neumann entropy of quantum subsystem.